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This manuscript reports on the combustion of powdered iron, for the purpose of utilizing it as an environmentally friendly circular energy carrier. The conducted research investigated the spectral emissivity and temperature of iron particles, burned either individually or in groups. Combustion experiments were conducted under high heating rates in an externally-heated drop tube furnace. The pressure was atmospheric and the axial temperature was nearly-constant at ~1350 K. The oxidizer gas contained 15-100% oxygen in nitrogen diluent. Iron particles were sieve-classified in the 44-53 µm range. Results showed that, depending on the oxygen concentration, and consequently the particle temperature, the average spectral emissivities of single burning particles varied between 0.18 and 0.46, in the 600-1000 nm wavelength range. Corresponding temperatures of single particles varied between 2300 K and 2800 K, increasing with increasing oxygen concentration in the gas. In the case of groups of iron particles burning in air at different particle number densities, average spectral emissivities were found to be in the range of 0.42-0.45, with the upper value associated with denser particle clouds. Corresponding peak temperatures of particle burning in groups were found to be in the range of 2160 K to 2100 K, with the lower value attributed to denser particle clouds.